論文

We theoretically investigate nonequilibrium spin fluctuations in a ferromagnet induced by a light pulse. Using a Lindblad equation consistent with the Landau-Lifshitz-Gilbert equation, we compute the autocorrelation function of magnetization. Our analysis reveals that this function comprises both thermal and nonequilibrium components. To examine the latter in detail, we introduce a Fano factor similar to nonequilibrium current noise in electronic circuits. We demonstrate that this factor encapsulates insights into the transfer of spin units to the environment. Our findings lay the groundwork for nonequilibrium spin noise spectroscopy, offering valuable insights into spin relaxation dynamics.

We present a novel method for generating spin currents using the gyromagnetic effect, a phenomenon discovered over a century ago. This effect, crucial for understanding the origins of magnetism, enables the coupling between various macroscopic rotational motions and electron spins. While higher rotational speeds intensify the effect, conventional mechanical rotations, typically, below 10,000 RPM, produce negligible results comparable to geomagnetic fluctuations, limiting applied research. Our studies demonstrate that spin current generation comparable to that of rare metals can be achieved through atomic rotations induced by GHz-range surface acoustic waves and the rotational motion of conduction electrons in metallic thin films with nanoscale gradient modulation of electrical conductivity. These effects, termed the acoustic gyromagnetic effect and the current-vorticity gyromagnetic effect, are significant in different contexts. The acoustic gyromagnetic effect is notable in high-conductivity materials like aluminum and copper, which are more abundant than conventional spintronics materials with strong spin–orbit interactions (SOIs). Conversely, the current-vorticity gyromagnetic effect requires a large conductivity gradient to produce current vorticity efficiently. This is achieved by using composition gradient structures from highly conductive metals to poorly conductive oxides or semiconductors. Consequently, unlike traditional strong-SOI materials, we can create highly efficient spin current generators with low energy dissipation due to reduced Joule loss.

Surface acoustic waves (SAWs) coupled to magnons have attracted much attention because they allow for the long-range transport of magnetic information that cannot be achieved by magnon alone. We employed pulsed laser interferometry to visualize the entire spatiotemporal dynamics of a SAW that travels on a nickel (Ni) thin film and is coupled to magnons. It was possible to trace the coupling-induced amplitude reduction and phase shift that occurs as the SAW propagates over a distance of 0.4 mm. The observed changes are consistent with results obtained from conventional radio-frequency transmission measurements, which probe the total SAW absorption due to magnon-phonon coupling. This result verifies that our method can accurately capture the spatiotemporal dynamics of a SAW coupled to magnons across the entire length of the sample. Additionally, we validated our time-resolved profiles by comparing them with theoretical results that take the echo wave due to reflection into account. The impact of the echo wave is significant even when it has propagated over a distance of the order of millimeters. Our imaging results highlight the visualization of the long-range propagation of the SAW coupled to magnons and offer more information about the surface vibration profiles in such devices.

We demonstrate a dual-comb vibrometer where the pulses of one frequency-comb are split into pulse pairs. We introduce a delay between the two pulses of each pulse pair in front of the sample, and after the corresponding two consecutive reflections at the vibrating sample surface, the initially introduced delay is cancelled by a modified Sagnac geometry. The remaining phase difference between the two pulses corresponds to the change in the axial position of the surface during the two consecutive reflections. The Sagnac geometry reduces the effect of phase jitter since both pulses propagate through nearly the same optical path (in opposite directions), and spurious signals are eliminated by time gating. We determine the amplitude of a surface vibration on a surface-acoustic-wave device with an axial precision of 4 pm. This technique enables highly accurate determination of extremely small displacements.

Precise measurements of the geometrical thickness of a sample and its refractive index are important for materials science, engineering, and medical diagnosis. Among the possible non-contact evaluation methods, optical interferometric techniques possess the potential of providing superior resolution. However, in the optical frequency region, the ambiguity in the absolute phase-shift makes it difficult to measure these parameters of optically thick dispersive materials with sufficient resolution. Here, we demonstrate that dual frequency-comb spectroscopy can be used to precisely determine the absolute sample-induced phase-shift by analyzing the data smoothness. This method enables simultaneous determination of the geometrical thickness and the refractive index of a planar sample with a precision of five and a half digits. The thickness and the refractive index at 193.414 THz (λ = 1550 nm) of a silicon wafer determined by this method are 0.5204737(19) mm and 3.475625(58), respectively, without any prior knowledge of the refractive index.

© 2018 by the author. This review focuses on several recent research activities regarding precise and fast polarization-sensitive terahertz time-domain spectroscopy systems for imaging purposes, and explains three interesting application examples. Owing to modulation techniques that have recently been developed for the evaluation of the instantaneous terahertz electric-field (E-field) vector, fast and precise terahertz polarization imaging becomes feasible. This terahertz technology enables high-resolution surface topography, precise understanding of the spatial E-field vector distribution of the focused terahertz pulse, and examination of strain-induced birefringence in polymeric materials. These examples constitute a new application area of terahertz photonics with emphasis on both fundamental optics and industrial applications.

By using intense terahertz(THz) monocycle pulses, nonlinear light-matter interaction in aligned semiconducting single-walled carbon nanotubes(SWNTs) embedded in a polymer film was investigated. THz electric-field-induced ultrafast Stark effect of onedimensional excitons in SWNTs was observed at room temperature, suggesting the potential functionality of SWNTs for high speed electro-optic devices operating at telecom wavelength with a THz bandwidth. When the peak electric field amplitude exceeds 200 kV/cm, the generation of excitons by the THz pump becomes prominent. The mechanism is described by the above-gap excitation of electrons and holes in SWNTs due to the impact excitation process induced by the intense THz electric field. © Springer Science+Business Media, LLC 2012.